When its drivers are set up properly, PSPP can produce output that looks very good indeed. The PostScript driver, suitably configured, can produce presentation-quality output. Here are a few guidelines for producing better-looking output, regardless of output driver. Your mileage may vary, of course, and everyone has different esthetic preferences.
init-string
setting. Try to get 132 columns; 160
might be better, but you might find that print that tiny is difficult to
read.
Try to strike a balance between character size and page width.